- Laiquendi, the Green-Elves of Ossiriand
- Druedain (like Ghan-buri-Ghan from Lord of the Rings)
- Easterlings (the people of Bor were faithful to the Elves, as opposed to the people of Ulfang)
- Ents and Maiar as mentioned, but to handle them with the sort of faithfulness Sil has shown so far would be difficult
- If you allowed peoples from outside Beleriand, the other houses of the dwarves, potentially other humans, or even proto-hobbits
That said, even the best of these are a bit marginal compared to the existing options; and one of the defining characteristics (in my view) of Sil is the fact that it hasn't expanded in the ramshackle way that *bands (particularly Zangband and its derivatives) have.
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